This study was to identify the structure of anger behavior that athletes illustrated in competitions. In order to achieve research purpose, 167 high school, college, and professional athletes responded to open questionnaires. Targeting 541 players, the structural validity of psychological measurement was verified. As a result of analyzing the sources of anger behaviors during matches, four factors of anger-out, anger-in, anger control, and anger-helplessness were deduced. Afterwards, the validity of 4 factor-model was verified through correlation analysis with trait anger and verification of group differences. That is, the level of trait anger had a positive relationship with expression of anger-out and anger-helplessness while it had a negative relationship with anger-in and anger-control. Especially, the behavioral aspect such as anger-helplessness is a structure that has not been found in other criteria of anger behavior and it reflects the uniqueness of sports situation. Based on such results, the significance of sport anger behavior and implications were discussed.